Interaction Effects on the Electronic Floquet Spectra: Excitonic Effects

מידע ביבליוגרפי
כותר: Interaction Effects on the Electronic Floquet Spectra: Excitonic Effects
Authors: Xiao, Teng, Huang, Tsan, Bao, Changhua, Sun, Zhiyuan
Publication Year: 2025
Collection: Condensed Matter
Physics (Other)
Quantum Physics
Subject Terms: Condensed Matter - Other Condensed Matter, Condensed Matter - Quantum Gases, Condensed Matter - Statistical Mechanics, Physics - Optics, Quantum Physics
תיאור: Floquet engineering of electronic states by light is a central topic in modern experiments. However, the impact of many-body interactions on the single-electron properties remains unclear in this non-equilibrium situation. We propose that interaction effects could be reasonably understood by performing perturbative expansion in both the pump field and the electron-electron interaction when computing physical quantities. As an example, we apply this approach to semiconductors and show analytically that excitonic effects, i.e., effects of electron-hole interaction, lead to dramatic corrections to the single-electron Floquet spectra even when the excitons are only virtually excited by the pump light. We compute these effects in phosphorene and monolayer MoS$_2$ for time- and angle-resolved photoemission spectroscopy (Tr-ARPES) and ultrafast optical experiments.
Document Type: Working Paper
Access URL: http://arxiv.org/abs/2505.07428
Accession Number: edsarx.2505.07428
Database: arXiv
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